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Calcium isotope selectivity was increased with polarized resonance ionization

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Research area:Atomic physicsAtomic and Molecular PhysicsAtomic and Molecular Physics, and Optics

What the study found

The study found that odd-even isotope selectivity in calcium can be increased using a laser resonance ionization scheme with linearly polarized light. The authors report suppression of abundant calcium-40 and selection of rare calcium-43, with a maximum reported separation coefficient of 9e3.

Why the authors say this matters

The authors conclude that this relatively simple method may be useful for increasing the selectivity of resonance ionization. They say it may have application to separating rare odd calcium isotopes, including calcium-43 for ion trapping in quantum information and calcium-41 for cosmology and biomedicine.

What the researchers tested

The researchers tested a laser resonance ionization J=0-1-0 transition scheme designed so that angular momentum selection rules could be applied using linearly polarized light. They varied the linear polarization angle using a half-waveplate and examined selectivity in both the resonance ionization process and spectroscopy at the Rydberg level transition.

What worked and what didn't

Setting the transition polarizations linearly orthogonal forbade excitation of the even isotopes in the electric dipole basis, while allowing excitation of the odd isotope. The abstract reports confirmed suppression of calcium-40 and selection of calcium-43 as the polarization angle was changed, and notes a final maximal selectivity of separation coefficient beta = 9e3, dependent on the hyperfine transition.

What to keep in mind

The reported maximum selectivity depended on the hyperfine transition. The abstract does not describe other limitations, experimental constraints, or performance outside the calcium isotopes studied.

Key points

  • Linearly polarized laser resonance ionization increased odd-even isotope selectivity in calcium.
  • Calcium-40 was suppressed and calcium-43 was selected by changing the polarization angle.
  • A half-waveplate was used to adjust the linear polarization.
  • The reported maximum separation coefficient was beta = 9e3.
  • The authors say the method may be useful for rare calcium isotope separation.

Disclosure

Research title:
Calcium isotope selectivity was increased with polarized resonance ionization
Authors:
Stephen R. Wells, Y. Iwata, Masabumi Miyabe, Shuichi Hasegawa
Institutions:
Japan Atomic Energy Agency, Japan Atomic Energy Agency, The University of Tokyo, The University of Tokyo, The University of Tokyo, The University of Tokyo
Publication date:
2026-02-24
OpenAlex record:
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AI provenance: This post was generated by gpt-5.4-mini (OpenAI). The original authors did not write or review this post.